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Which Way Does Stimulated Emission Go?

Abstract

Is it possible to form an image using light produced by stimulated emission? Here we study light scatter off an assembly of excited chromophores. Due to the Optical Theorem, stimulated emission is necessarily accompanied by excited state Rayleigh scattering. Both processes can be used to form images, though they have different dependencies on scattering direction, wavelength and chromophore configuration. Our results suggest several new approaches to optical imaging using fluorophore excited states.

Publication Details

Authors
Publication Type
Journal Article
Year of Publication
2021
Journal
Journal of Physical Chemistry A
Volume
125
Pagination
10667-10676